Collected Works of Lars Onsager: With Commentary by Hemmer P.C.

By Hemmer P.C.

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M o / . Cutul. 63 (1990) 319. R. Augustine, S. Tanielyan, S. Anderson, H. Yang, Chern. Commun. (1999) 1257. T. E. Davis, J. Curd. 148 (1994) I . T. E. Davis, J. Cutul. 152 (1995) 25. E. De Vos, F. P. F. A. Jacobs, Mucromol. Symp. 80 (1994) 157. B. Ogunwumi, T. Bein, Chem. Commun. (1997) 901. J. Sabater, A. C o m a , A. Domenech, V. Fomts, H. Garcia, Chem. Commun. (1997) 1285. J. Blum, D. Avnir, H. Schuhmann, Chemrech (1999) 32. J. Vankelecom, D. F. Parton, V. A. Jacobs, Angew. Chem. Int. Ed. Engl.

45 Ref a +=Heterogeneous reaction gives better results than the homogeneous one, even if this concerns sometimes only one subsrrate under specific conditions. OK=results are comparable to first run; +=better than in first run; -=worse than in first run. Type of heterogenization, following the classification in the text: cov =covalent attachment; ads = adsorption or ion pair formation; caps = encapsulation: trap =entrapment; SLP= supported liquid phase; aux =modification of an achiral heterogeneous catalyst with a chiral selector.

Based on the observed color change, this was tentatively explained for the hydrogenation with Rh(D1PAMP)(P/W)heteropolyacid-montmorilloniteby some partial reduction of the tungsten in the heteropolyacid. Lanthana was the only support that did not show this improvement, which was ascribed to its basic nature. 3 Encapsulation Encapsulating a TMC in the cages of a zeolite, for example, fully depends on the respective sizes of the complex and the cage in which it is held sterically to prevent leaching during reaction.

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