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Extra resources for Collected Works of Lars Onsager: With Commentary
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45 Ref a +=Heterogeneous reaction gives better results than the homogeneous one, even if this concerns sometimes only one subsrrate under specific conditions. OK=results are comparable to first run; +=better than in first run; -=worse than in first run. Type of heterogenization, following the classification in the text: cov =covalent attachment; ads = adsorption or ion pair formation; caps = encapsulation: trap =entrapment; SLP= supported liquid phase; aux =modification of an achiral heterogeneous catalyst with a chiral selector.
Based on the observed color change, this was tentatively explained for the hydrogenation with Rh(D1PAMP)(P/W)heteropolyacid-montmorilloniteby some partial reduction of the tungsten in the heteropolyacid. Lanthana was the only support that did not show this improvement, which was ascribed to its basic nature. 3 Encapsulation Encapsulating a TMC in the cages of a zeolite, for example, fully depends on the respective sizes of the complex and the cage in which it is held sterically to prevent leaching during reaction.